upto you how you do this... there are many methods for animé feel,
Zelda: Wind Waker is a definate cartoon feel and DragonballZ Saiyan (GC later this year) uses the same sort of techniques for some truely amazing graphics - but the cost was alot of polygons and no real textures as such.
however Bid For Power has an awesome Animé feel and does it all with simple textures
whatever you choose for the feel, it really is upto you as there are quite a few methods and techniques which all have thier own merits and pitfalls.
Tsu'va Oni Ni Jyuuko Fiori Sei Tau!
One block follows the suit ... the whole suit of blocks is the path ... what have you found?